南方科技大學是由中國廣東省領導和管理、深圳市舉全市之力創建的一所公辦創新型大學,目標是迅速建成國際化高水平研究型大學,建成中國重大科學技術研究與拔尖創新人才培養的重要基地……

                    南方科技大學以學分制、導師制、書院制為基礎,以人才培養的個性化、小班化、國際化為特色,通過為一流的人才培養體系,培養人格健全、基礎扎實、能力突出、具有國際視野、社會責任感、創新精神和實踐能力的高素質人才。

                    南科大已初步建成國際交流的平臺,與國際知名大學在人才培養、教學科研等方面達成合作協議,為學生開展境外交流學習。同時,學校積極與內地的多個機構開展全方位合作。

                    南方科技大學本科招生采用基于高考的綜合評價錄取模式,即高考成績占60%,我校自主組織的能力測試成績占30%(其中面談成績為5%),高中學業水平考試成績占10%,按考生“631”綜合成績排名從高到低錄取。綜合評價錄取模式由我校在2012年率先實施。

                    南科大教育基金會由理事會、監事會、秘書處組成。理事會是基金會的最高權力機構;監事會負責檢查財務和會計資料,監督理事會遵守法律和章程的情況;秘書處是基金會常設辦事機構,在理事會領導下負責基金會的日常工作。

                    學校黨委切實履行黨建工作職責,不斷強化班子建設和基層黨組織建設,充分發揮好黨委對學校各項工作的核心統領作用和各黨支部的戰斗堡壘作用,切實開展組織統戰和黨風廉政建設各項工作。學校高度重視群團組織建設,充分調動全體師生員工積極性,維護教職工的合法權益,推進學校民主管理,促進學校健康發展,全力營造齊心協力、團結向上、奮發有為的干事創業氛圍。

                    科研新聞

                    首頁 > 新聞動態 > 新聞信息 > 科研新聞 > Grubbs團隊...

                    科研新聞

                    Grubbs團隊在JACS上連續發表兩篇最新科研成果

                    2018-12-25 科研新聞

                            隨著深圳格拉布斯研究院(Shenzhen Grubbs Institute)在南科大的落成,2005年化學諾獎得主Grubbs教授已將其一部分重大科研項目轉移到南科大進行。近期,Grubbs團隊以深圳格拉布斯研究院為通訊單位連續在美國化學會化學頂級期刊J. Am. Chem. Soc.(IF 14.357)上發表兩篇論文,報道了他們在催化化學和合成化學領域取得的最新進展。


                    Grubbs教授與其在南科大的團隊

                            題為“Highly Active Platinum Catalysts for Nitrile and Cyanohydrin Hydration: Catalyst Design and Ligand Screening via High-Throughput Techniques”的論文講述了新型氰基水化催化劑的設計和發展應用過程。通過氰基水化反應合成酰胺是學術界和工業界制備各類酰胺化合物的主要途徑,因酰胺化合物是眾多醫藥和高分子材料的核心起始原料,產業需求量巨大,所以發展可高效實現氰基到酰胺轉化的催化劑成為過去幾十年合成化學家追求的重要目標之一。此項研究中,Grubbs團隊利用其發展新型催化劑的經驗,通過高通量配體篩選、催化劑合成、高通量反應條件優化的標準流程,發現了一系列新型氰基水化催化劑(下圖1)。與市售的氰基水化催化劑相比,Grubbs教授的催化劑在以下三方面取得了重大突破:1)催化效率達已知市售催化劑的數十倍;2)Grubbs催化劑在室溫即可實現氰基水化,而已知催化劑通常要在80-150 oC高溫才能實現該轉化;3)首次通過金屬催化的方式實現了α-羥基氰的水解,此前尚無催化劑可實現該轉化。作為Grubbs團隊成員,南科大研究助理教授陳波、化學系博士生李成程參與了該項研究工作。

                            Grubbs教授在過去十年中,進一步拓展了以他的名字命名的Grubbs催化劑,開發出具有高順式選擇性(Z-selective)以及立體保持選擇性(stereoretentive)的烯烴復分解催化劑。Grubbs團隊成員之一,格拉布斯研究院雙聘教授、化學系助理教授徐晨與Grubbs教授聯合發表題為“Concise Syntheses of Δ12-Prostaglandin J Natural Products via Stereoretentive Metathesis”的論文講述了應用該新型烯烴復分解催化劑高效實現Prostaglandins(前列腺素)類天然產物分子全合成的歷程。在哺乳動物組織中發現,Prostaglandins類分子具有廣泛的生物學功能和醫學應用。例如最近發現的Δ12-prostaglandin J家族的四個化合物(下圖2所示)具有顯著的抗癌活性,已經引起合成化學家的廣泛興趣。Grubbs團隊采用其最新發展的催化劑,通過“一鍋”立體保持的烯烴復分解策略,僅用7-8步(最長線性步驟)即分別完成了四個Δ12-prostaglandin J天然產物的全合成。到目前為止,這是已知的實現該類分子人工合成路線最短、最高效的方式。


                    左:圖1   右:圖2

                            上述研究工作得到了加州理工學院催化中心的大力支持,利用該中心的高通量篩選設備,Grubbs團隊完成了配體的篩選及反應條件優化。加州理工學院催化中心是Grubbs教授主持建立的旨在加快催化劑研發和反應條件優化、并加強不同研究領域之間交叉研究的科研平臺。值得一提的是,在Grubbs教授和格拉布斯研究院執行院長鄭智平的參與下,深圳格拉布斯研究院正在建設具備該類功能的催化中心,一旦落成,該中心將大大提高南科大在相關領域的研發能力,助力攻關重大科研課題。

                            Grubbs教授的研究方向集中在催化劑的設計、制備和篩選,以及催化劑在合成化學和高分子化學兩大領域的應用。

                    論文鏈接1:

                    https://pubs.acs.org/doi/10.1021/jacs.8b11667

                    論文鏈接2:

                    https://pubs.acs.org/doi/10.1021/jacs.8b12816

                     

                    供稿:深圳格拉布斯研究院

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